Volume One: 1961–1965
AlbumTracklist 228:15
CD 1
| 1 | Masquerade | 5:10 | |
| 2 | Funny Valentine | 3:29 | |
| 3 | Witchcraft | 2:24 | |
| 4 | Easy Living | 3:05 | |
| 5 | How Deep the Ocean | 3:09 | |
| 6 | Love for Sale | 2:54 | |
| 7 | Always | 2:59 | |
| 8 | How High the Moon | 2:29 | |
| 9 | Let Your Conscience Be Your Guide | 3:03 | |
| 10 | Never Let You Go | 2:43 | |
| 11 | You Don’t Know What Love Is | 3:53 |
CD 2
| 1 | Stubborn Kind of Fellow | 2:43 | |
| 2 | Pride & Joy | 2:35 | |
| 3 | Hitch Hike | 2:30 | |
| 4 | Get My Hands on Some Lovin’ | 2:25 | |
| 5 | Wherever I Lay My Hat | 2:14 | |
| 6 | Soldier’s Plea | 2:43 | |
| 7 | It Hurt Me Too | 2:43 | |
| 8 | Taking My Time | 2:27 | |
| 9 | Hello There Angel | 2:44 | |
| 10 | I’m Yours, You’re Mine | 1:55 |
CD 3
| 1 | You’ve Changed | 3:33 | |
| 2 | I Was Telling Her About You | 4:48 | |
| 3 | I Wonder | 3:44 | |
| 4 | I’ll Be Around | 4:09 | |
| 5 | Because of You | 3:33 | |
| 6 | I Don’t Know Why | 2:46 | |
| 7 | I’ve Grown Accustomed to Her Face | 3:31 | |
| 8 | When Your Lover Has Gone | 4:39 | |
| 9 | When I’m Alone I Cry | 3:47 | |
| 10 | If My Heart Could Sing | 3:22 |
CD 4
| 1 | Hello Broadway | 3:12 | |
| 2 | People | 3:15 | |
| 3 | The Party’s Over | 3:05 | |
| 4 | On the Street Where You Live | 2:26 | |
| 5 | What Kind of Fool Am I | 3:43 | |
| 6 | My Kind of Town | 2:38 | |
| 7 | The Days of Wine and Roses | 3:38 | |
| 8 | This Is the Life | 2:37 | |
| 9 | My Way | 2:55 | |
| 10 | Hello Dolly | 2:55 | |
| 11 | Walk on the Wild Side | 2:19 |
CD 5
| 1 | Once Upon a Time Marvin Gaye And Mary Wells | 2:33 | |
| 2 | Deed I Do Marvin Gaye And Mary Wells | 3:00 | |
| 3 | Until I Met You Marvin Gaye And Mary Wells | 3:26 | |
| 4 | Together Marvin Gaye And Mary Wells | 2:49 | |
| 5 | (I Love You) For Sentimental Reasons Marvin Gaye And Mary Wells | 2:35 | |
| 6 | The Late Late Show Marvin Gaye And Mary Wells | 2:41 | |
| 7 | After the Lights Go Down Low Marvin Gaye And Mary Wells | 2:53 | |
| 8 | Squeeze Me Marvin Gaye And Mary Wells | 2:38 | |
| 9 | What’s the Matter With You Baby Marvin Gaye And Mary Wells | 2:28 | |
| 10 | You Came a Long Way From St. Louis Marvin Gaye And Mary Wells | 2:51 |
CD 6
| 1 | You’re a Wonderful One | 2:43 | |
| 2 | How Sweet It Is (To Be Loved by You) | 2:59 | |
| 3 | Try It Baby | 2:52 | |
| 4 | Baby Don’t You Do It | 2:41 | |
| 5 | Need Your Lovin’ (Want You Back) | 2:19 | |
| 6 | One of These Days | 3:01 | |
| 7 | No Good Without You | 2:44 | |
| 8 | Stepping Closer to Your Heart | 2:42 | |
| 9 | Need Somebody | 2:52 | |
| 10 | Me and My Lonely Room | 2:52 | |
| 11 | Now That You’ve Won Me | 2:40 | |
| 12 | Forever | 2:20 |
CD 7
| 1 | Nature Boy | 2:51 | |
| 2 | Ramblin’ Rose | 2:51 | |
| 3 | Too Young | 3:48 | |
| 4 | Pretend | 2:49 | |
| 5 | Straighten Up and Fly Right | 2:24 | |
| 6 | Mona Lisa | 3:03 | |
| 7 | Unforgettable | 3:42 | |
| 8 | To the Ends of the Earth | 2:18 | |
| 9 | Sweet Lorraine | 2:48 | |
| 10 | It’s Only a Paper Moon | 2:26 | |
| 11 | Send for Me | 2:58 | |
| 12 | Calypso Blues | 4:06 |