Volume Two: 1966–1970
AlbumTracklist 274:12
CD 1
| 1 | I’ll Be Doggone | 2:49 | |
| 2 | Little Darling (I Need You) | 2:37 | |
| 3 | Take This Heart of Mine | 2:48 | |
| 4 | Hey Diddle Diddle | 2:30 | |
| 5 | One More Heartache | 2:42 | |
| 6 | Ain’t That Peculiar | 3:01 | |
| 7 | Night Life | 3:10 | |
| 8 | You’ve Been a Long Time Coming | 2:14 | |
| 9 | Your Unchanging Love | 3:14 | |
| 10 | You’re the One for Me | 3:25 | |
| 11 | I Worry ’Bout You | 3:24 | |
| 12 | One for My Baby (and One More for the Road) | 4:30 |
CD 2
| 1 | It Takes Two Marvin Gaye & Kim Weston | 2:57 | |
| 2 | I Love You, Yes I Do Marvin Gaye & Kim Weston | 2:19 | |
| 3 | Baby I Need Your Loving Marvin Gaye & Kim Weston | 3:10 | |
| 4 | It’s Got to Be a Miracle (This Thing Called Love) Marvin Gaye & Kim Weston | 3:28 | |
| 5 | Baby Say Yes Marvin Gaye & Kim Weston | 3:12 | |
| 6 | What Good Am I Without You Marvin Gaye & Kim Weston | 2:50 | |
| 7 | Till There Was You Marvin Gaye & Kim Weston | 2:24 | |
| 8 | Love Fell on Me Marvin Gaye & Kim Weston | 2:24 | |
| 9 | Secret Love Marvin Gaye & Kim Weston | 2:46 | |
| 10 | I Want You ’Round Marvin Gaye & Kim Weston | 2:22 | |
| 11 | Heaven Sent You I Know Marvin Gaye & Kim Weston | 3:00 | |
| 12 | When We’re Together Marvin Gaye & Kim Weston | 2:36 |
CD 3
| 1 | Ain’t No Mountain High Enough Marvin Gaye & Tammi Terrell | 2:29 | |
| 2 | You Got What It Takes Marvin Gaye & Tammi Terrell | 2:55 | |
| 3 | If I Could Build My Whole World Around You Marvin Gaye & Tammi Terrell | 2:21 | |
| 4 | Somethin’ Stupid Marvin Gaye & Tammi Terrell | 2:41 | |
| 5 | Your Precious Love Marvin Gaye & Tammi Terrell | 3:03 | |
| 6 | Hold Me Oh My Darling Marvin Gaye & Tammi Terrell | 2:47 | |
| 7 | Two Can Have a Party Marvin Gaye & Tammi Terrell | 2:14 | |
| 8 | Little Ole Boy, Little Ole Girl Marvin Gaye & Tammi Terrell | 2:41 | |
| 9 | If This World Were Mine Marvin Gaye & Tammi Terrell | 2:42 | |
| 10 | Sad Wedding Marvin Gaye & Tammi Terrell | 3:23 | |
| 11 | Give a Little Love Marvin Gaye & Tammi Terrell | 2:57 | |
| 12 | Oh How I’d Miss You Marvin Gaye & Tammi Terrell | 2:35 |
CD 4
| 1 | You | 2:27 | |
| 2 | Tear It On Down | 2:38 | |
| 3 | Chained | 2:40 | |
| 4 | I Heard It Through the Grapevine | 3:17 | |
| 5 | At Last (I Found a Love) | 2:40 | |
| 6 | Some Kind of Wonderful | 2:21 | |
| 7 | Loving You Is Sweeter Than Ever | 2:46 | |
| 8 | Change What You Can | 2:40 | |
| 9 | It’s Love I Need | 2:56 | |
| 10 | Every Now and Then | 3:07 | |
| 11 | You’re What’s Happening (In the World Today) | 2:22 | |
| 12 | There Goes My Baby | 2:25 |
CD 5
| 1 | Ain’t Nothing Like the Real Thing Marvin Gaye & Tammi Terrell | 2:16 | |
| 2 | Keep On Lovin’ Me Honey Marvin Gaye & Tammi Terrell | 2:31 | |
| 3 | You’re All I Need to Get By Marvin Gaye & Tammi Terrell | 2:51 | |
| 4 | Baby Don’tcha Worry Marvin Gaye & Tammi Terrell | 2:56 | |
| 5 | You Ain’t Livin’ Till You’re Lovin’ Marvin Gaye & Tammi Terrell | 2:49 | |
| 6 | Give In, You Just Can’t Win Marvin Gaye & Tammi Terrell | 2:35 | |
| 7 | When Love Comes Knocking at My Heart Marvin Gaye & Tammi Terrell | 2:30 | |
| 8 | Come On and See Me Marvin Gaye & Tammi Terrell | 2:27 | |
| 9 | I Can’t Help but Love You Marvin Gaye & Tammi Terrell | 2:48 | |
| 10 | That’s How It Is (Since You’ve Been Gone) Marvin Gaye & Tammi Terrell | 3:01 | |
| 11 | I’ll Never Stop Loving You Baby Marvin Gaye & Tammi Terrell | 3:22 | |
| 12 | Memory Chest Marvin Gaye & Tammi Terrell | 2:56 |
CD 6
| 1 | Too Busy Thinking About My Baby | 2:59 | |
| 2 | This Magic Moment | 2:43 | |
| 3 | That’s the Way Love Is | 3:45 | |
| 4 | The End of Our Road | 2:53 | |
| 5 | Seek and You Shall Find | 3:42 | |
| 6 | Memories | 2:48 | |
| 7 | Only a Lonely Man Would Know | 3:04 | |
| 8 | It’s a Bitter Pill to Swallow | 3:14 | |
| 9 | More Than a Heart Can Stand | 2:58 | |
| 10 | Try My True Love | 2:58 | |
| 11 | I Got to Get to California | 2:53 | |
| 12 | It Don’t Take Much to Keep Me | 2:43 |
CD 7
| 1 | Good Lovin’ Ain’t Easy to Come By Marvin Gaye & Tammi Terrell | 2:28 | |
| 2 | California Soul Marvin Gaye & Tammi Terrell | 2:50 | |
| 3 | Love Woke Me Up This Morning Marvin Gaye & Tammi Terrell | 2:31 | |
| 4 | This Poor Heart of Mine Marvin Gaye & Tammi Terrell | 2:41 | |
| 5 | I’m Your Puppet Marvin Gaye & Tammi Terrell | 2:59 | |
| 6 | The Onion Song Marvin Gaye & Tammi Terrell | 2:59 | |
| 7 | What You Gave Me Marvin Gaye & Tammi Terrell | 2:44 | |
| 8 | Baby I Need Your Loving Marvin Gaye & Tammi Terrell | 3:12 | |
| 9 | I Can’t Believe You Love Me Marvin Gaye & Tammi Terrell | 2:44 | |
| 10 | How You Gonna Keep It (After You Get It) Marvin Gaye & Tammi Terrell | 2:52 | |
| 11 | More, More, More Marvin Gaye & Tammi Terrell | 2:29 | |
| 12 | Satisfied Feelin’ Marvin Gaye & Tammi Terrell | 2:54 |
CD 8
| 1 | Gonna Give Her All the Love I’ve Got | 3:22 | |
| 2 | Yesterday | 3:26 | |
| 3 | Groovin’ | 2:57 | |
| 4 | I Wish It Would Rain | 2:50 | |
| 5 | That’s the Way Love Is | 3:44 | |
| 6 | How Can I Forget | 2:04 | |
| 7 | Abraham, Martin and John | 4:30 | |
| 8 | Gonna Keep On Tryin’ Till I Win Your Love | 2:46 | |
| 9 | No Time for Tears | 2:26 | |
| 10 | Cloud Nine | 3:19 | |
| 11 | Don’t You Miss Me a Little Bit Baby | 2:14 | |
| 12 | So Long | 2:30 |