Early Years (1963–1968)
AlbumTracklist 79:27
| 1 | Aurora (mono) The Squires | 2:10 | |
| 2 | The Sultan (mono) The Squires | 2:35 | |
| 3 | I Wonder (mono) The Squires | 2:23 | |
| 4 | Mustang (instrumental) (mono) The Squires | 2:25 | |
| 5 | I’ll Love You Forever (mono) The Squires | 3:24 | |
| 6 | (I’m a Man and) I Can’t Cry (mono) The Squires | 2:34 | |
| 7 | Hello Lonely Woman (previously unreleased version) Neil Young & Comrie Smith | 3:59 | |
| 8 | Casting Me Away From You Neil Young & Comrie Smith | 2:15 | |
| 9 | There Goes My Babe Neil Young & Comrie Smith | 2:26 | |
| 10 | Sugar Mountain (previously unreleased demo version) (mono) | 2:43 | |
| 11 | Nowadays Clancy Can’t Even Sing (demo version) (mono) | 3:05 | |
| 12 | Runaround Babe (mono) | 2:38 | |
| 13 | The Ballad of Peggy Grover (mono) | 2:48 | |
| 14 | The Rent Is Always Due (mono) | 2:54 | |
| 15 | Extra, Extra (mono) | 2:44 | |
| 16 | Flying on the Ground Is Wrong (mono) | 3:11 | |
| 17 | Burned (mono) Buffalo Springfield | 2:18 | |
| 18 | Out of My Mind (mono) Buffalo Springfield | 3:08 | |
| 19 | Down, Down, Down (previously unreleased version) (mono) | 2:14 | |
| 20 | Kahuna Sunset (mono) Buffalo Springfield | 2:54 | |
| 21 | Mr. Soul (mono) Buffalo Springfield | 2:46 | |
| 22 | Sell Out (mono) Buffalo Springfield | 1:43 | |
| 23 | Down to the Wire (mono) Buffalo Springfield | 2:31 | |
| 24 | Expecting to Fly Buffalo Springfield | 3:47 | |
| 25 | Slowly Burning (instrumental) | 3:01 | |
| 26 | One More Sign | 2:04 | |
| 27 | Broken Arrow Buffalo Springfield | 6:17 | |
| 28 | I Am a Child Buffalo Springfield | 2:18 |